Carracedo Pérez, MaríaPrieto López, CristinaBlanco Vales, MaríaMagariños Ferro, BeatrizLópez Iglesias, ClaraGarcía González, Carlos A.2025-11-112025-11-112025-08-30Carracedo-Pérez, M., Prieto, C., Blanco-Vales, M., Magariños, B., López-Iglesias, C., & García-González, C. A. (2025). Breathing green: Sustainable approaches for the reuse of FFP2 facemasks. Journal of Environmental Chemical Engineering, 13(5), 118991. 10.1016/j.jece.2025.1189912213-2929https://hdl.handle.net/10347/43700Facemasks are essential components in healthcare environments, but their disposal represents a significant environmental concern. This study proposes an optimized sterilization treatment for the reprocessing of electrostatic filter (EF) and mechanical filter (MF) facemasks using supercritical carbon dioxide (scCO2) and hydrogen peroxide, achieving a Sterility Assurance Level (SAL) of 10−6 in microbial load. The performance of the facemasks was evaluated after 1, 5, and 10 cycles and compared with those subjected to ethylene oxide and to γ-rays sterilization procedures, in terms of filtration efficiency, breathability, electrostatic charges of the filters, and of mechanical properties of the elastic bands. Structural and chemical changes were characterized using SEM and FTIR. The findings demonstrated that scCO2 treatment induced electrostatic charges in the MF, improving their filtration efficiency. The supercritical treatment also preserved the chemical and structural integrity of both types of filters. Results underscore the effectiveness of the scCO2 method as a viable and sustainable alternative to conventional sterilization methods.eng© 2025 The Author(s). Published by Elsevier Ltd. This is an open access article under the CC BY license (http://creativecommons.org/licenses/by/4.0/).Attribution 4.0 Internationalhttp://creativecommons.org/licenses/by/4.0/Mechanical filterElectrostatic filterSterilizationSupercritical fluid technologyGreen processingjournal article10.1016/j.jece.2025.118991open access