Tunnel conduction in epitaxial bilayers of ferromagnetic LaCoO3/La2/3Sr1/3MnO3 deposited by a chemical solution method

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ISSN: 1944-8244
E-ISSN: 1944-8252

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American Chemical Society
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We report magnetic and electronic transport measurements across epitaxial bilayers of ferromagnetic insulator LaCoO3 and half-metallic ferromagnet La2/3Sr1/3MnO3 (LCO/LSMO: 3.5 nm/20 nm) fabricated by a chemical solution method. The I–V curves at room temperature and 4K measured with conducting atomic force microscopy (CAFM) on well-defined patterned areas exhibit the typical features of a tunneling process. The curves have been fitted to the Simmons model to determine the height (φ) and width (s) of the insulating LCO barrier. The results yield φ = 0.40 ± 0.05 eV (0.50 ± 0.01 eV) at room temperature (4K) and s = 3 nm, in good agreement with the structural analysis. Our results demonstrate that this chemical method is able to produce epitaxial heterostructures with the quality required for this type of fundamental studies and applications.

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“This document is the Accepted Manuscript version of a Published Article that appeared in final form in [ACS Applied Materials & Interfaces], copyright © [ 2014 American Chemical Society]. To access the final published article, see DOI: 10.1021/am506259p”

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Lucas, I., Vila-Fungueiriño, J. M., Jiménez-Cavero, P., Rivas-Murias, B., Magén, C., Morellón, L., & Rivadulla, F. (2014). Tunnel Conduction in Epitaxial Bilayers of Ferromagnetic LaCoO3/La2/3Sr1/3MnO3 Deposited by a Chemical Solution Method. ACS Applied Materials & Interfaces, 6(23), 21279-21285. https://doi.org/10.1021/am506259p

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The authors aknowledge the support to this work from Spanish Ministry of Science through project Nos. MAT2011-28532-C03-02, MAT2013-44673-R, and MAT2011-27553-C02 including FEDER funding, the Aragón Regional Government (Project No. E26), ERC-StG-259082(2DTHERMS) and Xunta de Galicia (2012-CP071). Jose Manuel Vila-Fungueiriño aknowledges MINECO of Spain for support through the FPI program, and Irene Lucas and Cesar Magen aknowledge Fundación Aragonesa para la I+D for support through ARAID program

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